The aim of this work was to explore the relationship between dark triad and five-factor personality model with work and organizational attitudes: job satisfaction, organizational commitment, and job involvement. The research was conducted on 217 employees of several large organizations from the Karlovac and Varaždin counties. Personality traits were examined with the Dark Triad Questionnaire and the Five-Factor Personality Questionnaire, while different groups of job attitudes were examined with the Job Satisfaction Questionnaire, the Organizational Commitment Questionnaire, and the Job Involvement Scale. Overall job satisfaction and its components have a positive correlation with extraversion, agreeableness, conscientiousness and openness, and negative with Machiavellianism, narcissism, psychopathy and neuroticism. The mentioned personality traits proved to be significant predictors of certain components of job satisfaction. Organizational commitment and its components correlate positively with Machiavellianism, extraversion, agreeableness, conscientiousness, and openness. Significant predictors are conscientiousness for organizational and affective commitment and Machiavellianism for rational commitment. Job involvement correlates positively with narcissism, extraversion, agreeableness, conscientiousness and openness, and negatively with psychopathy and neuroticism. Significant predictors are narcissism, psychopathy, agreeableness and conscientiousness. The examined attitudes towards work and organization are predicted and explained by personality traits of the five-factor model much better than dark triad, although job satisfaction and some of its components are additionally explained by the inclusion of the dimensions of the dark triad.